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Advances in Chemical Physics [Vol 10 - Molecular Beams] by I. Prigogine

By I. Prigogine

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The only cases for which Eq. (36) has been solved are those in which the scattering geometry permits several simplifications. In the first of thesez6 it is possible to carry out the analysis by assuming that the source of the beam is a point located at the intersection of lines drawn from the edge of the beam at the detector plane through the edge of the entrance aperture of the scattering chamber. It can be shown that this model can be obtained as a special case of Eq. (36). The actual analysis is similar to that for a parallel beam, and in the limit of very small beam divergence the two treatments become identical.

Cambridge. Massachusetts CONTENTS I . Introduction ................................................... I1 Fundamental Concepts ......................................... 111 Analysis ...................................................... A General Features of Elastic Scattering ........................ B Detailed Analysis of Scattering Experiments ................... 1 Classical Analysis for Central Forces ...................... 2 . Scattering by a Non-Central Force ........................ 3. Background Scattering ..................................

6. E. U. Condon and G. H. Shortley, The Theory of Atomic Spectra, Cambridge University Press, New York, 1951,p. 6Off. 7. Dalgarno and A. E. Kingston, Proc. Phys. Sac. (London), A73, 455 (1959). 8. R. Sternheimer, Phys. , %, 951 (1954). 9. Dalgarno, Advan. Ground-state polarizabilities of the helium isoelectronic sequence have been calculated, using the fully coupled Hartree-Fock approximation, by A. Dalgarno and J. M. , Proc. Phys. ,77,673 (1961). The method has recently been extended to the beryllium sequence by A.

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